Exciton Dynamics in Lead Halide Perovskite Nanocrystals: Recombination, Dephasing and Diffusion

di Bernhard Johann Bohn (Autore)

Springer Nature Switzerland AG, 2022

Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission.   In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as theactive layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.

• Autore: Bernhard Johann Bohn
• Editore: Springer Nature Switzerland AG
• Collana: Springer Theses
• Anno: 2022
• Rilegatura: Paperback / softback
• Pagine: 152 p.
• Dimensioni: 235 x 155 mm
• EAN: 9783030709426

Testo in English